Advances in Organometallic Chemistry, 7 by F G A Stone; Robert West

By F G A Stone; Robert West

ADVANCES ORGANOMETALLIC CHEMISTRY V 7.

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With the great variety of polyhalogenated compounds, containing varying numbers of fluorine, chlorine, and bromine atoms; and with the heterogeneity of the several reaction systems ; and with a variety of metals in place of lithium, it is to be expected that no single mechanism may be operating. One simple intermediate that is reasonable is tetralithiopropyne. Another possible intermediate is trimethylsilyllithium. This is postulated because of the reactions of R3SiLi compounds with some polyhalogenated types of compounds.

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A. G. ), p. 321. Academic Press, New York, 1962. 32. Ingham, R. , in “Introduction to Organotin Chemistry” (A. K. ), M. Dekker, New York, 1968. 33. Ingham, R. , Rosenberg, S. , Chem. Rew. 60, No. 5,459 (1960). 34. Jones, R. , Org. Reactions6, 339 (1951). 35. Jones, R. , Chem. Rew. 54, No. 5, 835 (1954). 36. Kharasch, M. , “ Grignard Reactions of Non-metallic Substances,” p. 95. Prentice-Hall, Englewood Cliffs, New Jersey, 1954. 37. Leeper, R. , Chem. Rev. 54, No. 1, 101 (1954). 38. LeMahieu, R.

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